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Technically, yes—and you may have some successful growth—but this isn’t the ideal way to fill in sparse areas. By clearing leaves and debris, amending the soil, and aerating it properly before you lay the seeds, you’re providing the most ideal conditions for them to germinate.

Aeration can level your lawn if the issue is minor soil compaction, so it can help smooth things out if your yard is bumpy from foot traffic or vehicle traffic. However, it won’t slope your yard. If you have small areas where water seems to pool after precipitation, aeration could help, but larger issues with improperly sloped lawns and problems leading to foundation leaks or structural damage will require more comprehensive solutions.

There are plenty of products to help green up your grass. Try an iron supplement spray or fertilizer that is rich in nitrogen. You can also apply a thin layer of compost on top of your lawn at the beginning of spring to give the grass a nutrition boost, which helps it achieve that bright color you are looking for. 

To prepare your lawn for core aeration, water it the day before you aerate. (Alternatively, you can wait until it rains and aerate the following day.) Aerating after watering or a rainy day will make the process easier since you can penetrate moist soil better than dry soil. You should also flag your sprinklers so that you don’t accidentally hit them while aerating. If you have a lot of thatch buildup in your yard, you might need to dethatch your lawn before aerating as well.